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2019年11月28日

【期刊论文】investigation of charge injection and transport behaviour in multilayer structure consisted of ferromagnetic metal and organic polymer under external fields

hua zhao, wei-feng meng

superlattices and microstructures,2017,110((2017&):31-48

2017年07月15日

in this paper a five layer organic electronic device with alternately placed ferromagnetic metals and organic polymers: ferromagnetic metal/organic layer/ferromagnetic metal/organic layer/ferromagnetic metal, which is injected a spin-polarized electron from outsides, is studied theoretically using one-dimensional tight binding model hamiltonian. we calculated equilibrium state behavior after an electron with spin is injected into the organic layer of this structure, charge density distribution and spin polarization density distribution of this injected spin-polarized electron, and mainly studied possible transport behavior of the injected spin polarized electron in this multilayer structure under different external electric fields. we analyze the physical process of the injected electron in this multilayer system. it is found by our calculation that the injected spin polarized electron exists as an electron-polaron state with spin polarization in the organic layer and it can pass through the middle ferromagnetic layer from the right-hand organic layer to the left-hand organic layer by the action of increasing external electric fields, which indicates that this structure may be used as a possible spin-polarized charge electronic device and also may provide a theoretical base for the organic electronic devices and it is also found that in the boundaries between the ferromagnetic layer and the organic layer there exist induced interface local dipoles due to the external electric fields.

five layer organic electronic structure, electron-polaron transport, spin polarization, injection of

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2018年10月18日

【期刊论文】the study of charge injection and spin polarization in ferromagnetic metal–polymer–ferromagnetic metal structure

hua zhao, zhong-wang liu,, shao-bo chen, liu-an chang

physica b,2014,450(1):111-115

2014年05月10日

by using extended ssh hamiltonian plus long-range electron correlation hamiltonian model, we calculated charge injection and spin polarization in a ferromagnetic metal/polymer/ferromagnetic metal structure. we adjust relative chemical potential between the ferromagnetic materials and the polymer to control charge transfer. it is found that when spin orientations of two ferromagnetic materials are parallel to each other, spin-polarized single polaron can be formed in the polymer, but when the spin orientations of two ferromagnetic materials are antiparallel to each other, bipolaron is formed and that spin polarization is found to be zero inside the polymer. the influence of the long-range electronic correlation on these polarons in the polymer is discussed

spin polarization,, charge injection,, long-range electron correlation,, bipolaron,, spin splitting

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2011年04月18日

【期刊论文】long-range correlation energies, off-diagonal interactions and correlation hamiltonian for π electronic systems

赵铧, hua zhao, 赵铧, hua zhao

j supercond nov magn (2010)23: 1173-1175,-0001,():

-1年11月30日

a general formula of the long-range correlation energy ec for the π electron systems is given, which includes diagonal interactions and off-diagonal interactions and we put forward to a correlation hamiltonian at the first time. it is found that the effects of the off-diagonal interactions w and x on the correlation energies are opposite. the effect of w is to increase the correlation energies, but the effect of x is being counteracted by the integral term j due to |x|~|j |. the long-range correlation energies decrease with increasing the screening effect. at normal screening, the influence of w on the correlation energies can be neglected.

long-range correlation energies • off-diagonal interactions • correlation hamiltonian • π electronic systems

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2011年04月18日

【期刊论文】long-range correlation energies calculations for excited states ofπ electronic systems

赵铧, hua zhao

physica b405(2010)4450-4452,-0001,():

-1年11月30日

a general formula of long-range electron correlation energy in excited states ofπelectron systems is presented for the first time. effect of excited states upon the long-range electron correlations, which are related to problems of exciton and polaron, is discussed. it is found that because charge density distributions are different for removal (addition) of an electron from (into) π electron system, the correlation energies of electron-type polaron and hole-type polaron are not the same even when the system tends to infinity.

excited states long-range electron correlation energy electron-hole asymmetryπelectron systems

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2011年04月18日

【期刊论文】correlation energies calculations for poly (p-phenylenevinylene) (ppv) chains

赵铧, hua zhao

journal of theoretical and computational chemistry vol. 8, no.5(2009)881-886,-0001,():

-1年11月30日

the present study calculates correlation energies of the different length poly(pphenylenevinylene) (ppv) units using the formula recently developed for π conjugated polymers, and analyzes the correlation energies from the phenylene unit and the vinylene unit in single and three ppv unit cells as well as the effect of the correlation energies on the band energy gap of the ppv. the present method avoids the complicated numerical computations about the correlation effects for the π electronic conjugated molecule systems with large unit cells.

long-range correlation, long-range correlation energies, ppv.,

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    重庆大学,重庆

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